A GGCT fluorogenic probe: design, synthesis and application to cancer-related cells.

نویسندگان

  • Taku Yoshiya
  • Hiromi Ii
  • Shugo Tsuda
  • Susumu Kageyama
  • Tatsuhiro Yoshiki
  • Yuji Nishiuchi
چکیده

Cancer-related γ-glutamyl cyclotransferase (GGCT) specifically converts γ-glutamyl amino acids (γ-Glu-Xaa) into pyroglutamate and the corresponding amino acids (Xaa). Here we report a novel GGCT fluorogenic probe "LISA-101" containing a masked O-acylated fluorophore "resorufin" on the side chain of the P amino acid (Xaa). Upon GGCT treatment, the P amino acid was liberated and spontaneously released the intact fluorophore. Thus, the fluorescence was regained. LISA-101 will expand the strategies for cancer studies.

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عنوان ژورنال:
  • Organic & biomolecular chemistry

دوره 13 11  شماره 

صفحات  -

تاریخ انتشار 2015